Nuggets: Original Artyfacts from the First Psychedelic Era by Various
It's a compilation of psych-garage rock bands from '65-'68. Mainly obscure and unheard of artists. But great nonetheless.
A sample: http://www.youtube.com/watch?v=oA2WUJwA0tY
another compilation album, haha.
Relics by Pink Floyd
Great psychedelic stuff also! mid to late sixties.http://www.youtube.com/watch?v=9NqY2aEYJ4c
of course it's not the best of my library, just what I'm listening to ATM!
enjoy... or not